After the turn of the 21st century, Smith's acting appearances became more sporadic. Among her most recent film appearances were in the 2006 film Loveless in Los Angeles, a romantic comedy movie that took place behind the scenes of a reality dating show, and a featured role, that of Kitty Carloff, in the 2007 film The Seduction of Dr. Fugazzi, which also starred Faye Dunaway.